The field of nanocatalysis has gained significant attention in the last decades due to the numerous industrial applications of nanosized catalysts. Size, shape, structure, and composition of the nanoparticles (NPs) are the parameters that can affect the reactivity, selectivity and stability of nanocatalysts. Therefore, understanding how these parameters affect the catalytic properties of these systems is required in order to engineer them with a given desired performance. It is also important to gain insight into the structural evolution of the NP catalysts under different reaction conditions to design catalysts with long durability under reaction condition. In this dissertation a synergistic combination of in situ, ex situ and operando state-of-the art techniques have allowed me to explore a variety of parameters and phenomena relevant to nanocatalysts by systematically tuning the NP size, chemical state, composition and chemical environment.
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Roldan Cuenya, Beatriz
Doctor of Philosophy (Ph.D.)
College of Sciences
Length of Campus-only Access
Doctoral Dissertation (Open Access)
Ahmadi, Mahdi, "Size, Shape, Composition and Chemical state effects in nanocatalysis" (2016). Electronic Theses and Dissertations. 5096.