Title

Microstructure and ionic conductivity of alternating-multilayer structured Gd-doped ceria and zirconia thin films

Authors

Authors

Y. G. Wang; L. A. An; L. V. Saraf; C. M. Wang; V. Shutthanandan; D. E. McCready;S. Thevuthasan

Comments

Authors: contact us about adding a copy of your work at STARS@ucf.edu

Abbreviated Journal Title

J. Mater. Sci.

Keywords

OXIDE FUEL-CELLS; Materials Science, Multidisciplinary

Abstract

Multilayer thin film of Gd-doped ceria and zirconia have been grown by sputter-deposition on alpha-Al2O3 (0001) substrates. The films were characterized using X-ray diffraction (XRD), atomic force microscopy (AFM), X-ray photoelectron spectroscopy (XPS), and transmission electron microscopy (TEM). The Gd-doped ceria and zirconia layers had the fluorite structure and are highly textured such that the (111) plane of the films parallel to the (0001) plane of the alpha-Al2O3. The epitaxial relationship can be written as (111)(ZrO2/CeO)2//(0001)Al2O3 and [11-2](ZrO2/CeO2)// [-2110](Al2O3), respectively. The absence of Ce3+ features in the XPS spectra indicates that the Gd-doped ceria films are completely oxidized. The ionic conductivity of this structure shows great improvement as compared with that of the bulk crystalline material. This research provides insight on designing of material for low temperature electrolyte applications.

Journal Title

Journal of Materials Science

Volume

44

Issue/Number

8

Publication Date

1-1-2009

Document Type

Article

Language

English

First Page

2021

Last Page

2026

WOS Identifier

WOS:000264485100014

ISSN

0022-2461

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