Title

Electron Transport in Polymer-Derived Amorphous Silicon Oxycarbonitride Ceramics

Authors

Authors

Y. S. Wang; T. Jiang; L. G. Zhang;L. A. An

Comments

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Abbreviated Journal Title

J. Am. Ceram. Soc.

Keywords

CARBONITRIDE CERAMICS; LOCALIZED STATES; HIGH-TEMPERATURE; FILMS; CONDUCTION; CONVERSION; PRECURSOR; NITRIDE; Materials Science, Ceramics

Abstract

The electron transport behavior of polymer-derived amorphous silicon oxycarbonitride ceramics is studied by measuring their temperature-dependent electrical conductivities. The experimental results are analyzed using theoretical models. The results reveal that the materials exhibit three conduction mechanisms: conduction in extended states, conduction in band tails, and conduction in localized states. Particularly, it is found that in a low-temperature regime, the conduction of the materials follows a band tail hopping mechanism, rather than the previously assumed variable range hopping mechanism. The results also reveal that energy gaps such as E(C)-E(F) and E(C)-E(A) decrease with increasing pyrolysis temperature.

Journal Title

Journal of the American Ceramic Society

Volume

92

Issue/Number

7

Publication Date

1-1-2009

Document Type

Article

Language

English

First Page

1603

Last Page

1606

WOS Identifier

WOS:000267426500038

ISSN

0002-7820

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