Title

Photostability of a series of two-photon absorbing fluorene derivatives

Authors

Authors

K. D. Belfield; M. V. Bondar; O. V. Przhonska;K. J. Schafer

Comments

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Abbreviated Journal Title

J. Photochem. Photobiol. A-Chem.

Keywords

fluorene derivatives; photochemical quantum yield; photostability; photooxidation; EXCITATION; PHOTON; DYES; Chemistry, Physical

Abstract

The photochemical stability of a series of two-photon absorbing (TPA) fluorene derivatives was investigated in air- and N-2-saturated acetonitrile (ACN) at room temperature. The quantum yields of the photoreactions, Phi, were determined at various concentrations of the fluorene derivatives, oxygen concentration of the solvent, and irradiation wavelength. The absorption and fluorescence spectra of the photoproducts, corresponding to different excitation conditions, were analyzed. Photooxidation and electron transfer processes are proposed as photobleaching mechanisms for the fluorene derivatives in ACN. The relatively low photochemical quantum yields (Phi similar to 10(-4)) make the derivatives particularly promising for linear and nonlinear optical applications. (C) 2004 Elsevier B.V. All rights reserved.

Journal Title

Journal of Photochemistry and Photobiology a-Chemistry

Volume

162

Issue/Number

2-3

Publication Date

1-1-2004

Document Type

Article

Language

English

First Page

489

Last Page

496

WOS Identifier

WOS:000220468500032

ISSN

1010-6030

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