Title

Strong two-photon absorption at telecommunications wavelengths in nickel bis(dithiolene) complexes

Authors

Authors

J. Y. Cho; S. Barlow; S. R. Marder; J. Fu; L. A. Padilha; E. W. Van Stryland; D. J. Hagan;M. Bishop

Comments

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Abbreviated Journal Title

Opt. Lett.

Keywords

OPTICAL NONLINEARITIES; DITHIOLENE COMPLEXES; PHASE CONJUGATION; ORGANIC-MOLECULES; LIQUID-CRYSTALS; CROSS-SECTIONS; SINGLE-BEAM; 1550; NM; ENHANCEMENT; ACCEPTOR; Optics

Abstract

The two-photon absorption spectrum of a nickel bis(dithiolene) complex with extended conjugation and pi-donor substitution is measured by using Z-scan and pump-probe techniques with femtosecond pulses over the spectral range from 1.20 to 1.58 mu m, which includes much of the telecommunications range. The peak two-photon cross section of over 5000 GM (1 GM = 10(-50) cm(4)s photon(-1) molecule(-1)) occurs at similar to 1.24 mu m, with significant two-photon absorption (> 440 GM) throughout the spectral range examined. (c) 2007 Optical Society of America.

Journal Title

Optics Letters

Volume

32

Issue/Number

6

Publication Date

1-1-2007

Document Type

Article

Language

English

First Page

671

Last Page

673

WOS Identifier

WOS:000244726900030

ISSN

0146-9592

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