Title

Comparison of BEA, USY and ZSM-5 for the quantitative extraction of polycyclic aromatic hydrocarbons from water samples

Authors

Authors

A. A. Costa; W. B. Wilson; H. Y. Wang; A. D. Campiglia; J. A. Dias;S. C. L. Dias

Comments

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Abbreviated Journal Title

Microporous Mesoporous Mat.

Keywords

Zeolite; Water; Extraction; Polycyclic aromatic hydrocarbons; Adsorption; LOW-COST ADSORBENTS; MOLECULARLY IMPRINTED POLYMER; GRANULAR ACTIVATED; CARBON; LAYERED DOUBLE HYDROXIDES; HEAVY-METALS; ZEOLITE-BETA; WASTE-WATER; ADSORPTION; REMOVAL; SORPTION; Chemistry, Applied; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary

Abstract

The physicochemical properties of three commercial zeolites - namely BEA, USY and ZSM-5 - are compared for the water removal of 15 PAHs included in the US EPA priority pollutants list. The best percentages of extraction were obtained with BEA and varied from 85.2 +/- 1.7% (benzo[g,h,i]perylene) to 99.6 +/- 1.1% (pyrene). The correlation of physicochemical properties to the percentages of extraction suggests that the predominant factor for a successful extracting performance is the adsorption of PAHs to the external surface of the extracting material. This process is facilitated by relatively large total pore volumes, large average pore diameters and a homogeneous distribution of Lewis acid sites. The presence of the latter enhances extraction performance via pi-electron interactions with the aromatic rings of the PAH. (C) 2011 Published by Elsevier Inc.

Journal Title

Microporous and Mesoporous Materials

Volume

149

Issue/Number

1

Publication Date

1-1-2012

Document Type

Article

Language

English

First Page

186

Last Page

192

WOS Identifier

WOS:000296933200025

ISSN

1387-1811

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