Title
Sol-Gel Synthesis And Phase Evolution Behavior Of Sterically Stabilized Nanocrystalline Zirconia
Keywords
Hydroxypropyl cellulose; Nanocry stalline; Sol-gel; Steric-stabilization; XPS; Zirconia
Abstract
Nanocrystalline as well as submicron sized, non-agglomerated, spherical ZrO2 particles have been successfully synthesized using the sol-gel technique utilizing hydroxypropyl cellulose (HPC) as a polymeric steric stabilizer. The effect of various parameters such as the ratio of molar concentration of water and alkoxide (R), the molar concentration [HPC] and the molecular weight (MWHPC) of HPC polymer as well as the calcination temperature on ZrO2 nanocrystallites size and their phase evolution behavior is systematically studied. The phase evolution behavior of nanocry stalline ZrO2 is explained and correlated with the adsorption behavior of HPC polymer on ZrO2 nanoparticles surface, which is observed to be a function of R, [HPC], MWHPC and the calcination temperature. Optimum synthesis parameters for obtaining 100% tetragonal phase in nanocry stalline ZrO2 are identified for the present sol-gel method of synthesizing nanoparticles.
Publication Date
6-1-2003
Publication Title
Journal of Sol-Gel Science and Technology
Volume
27
Issue
2
Number of Pages
119-136
Document Type
Article
Personal Identifier
scopus
DOI Link
https://doi.org/10.1023/A:1023790231892
Copyright Status
Unknown
Socpus ID
0038605846 (Scopus)
Source API URL
https://api.elsevier.com/content/abstract/scopus_id/0038605846
STARS Citation
Shukla, S.; Seal, S.; and Vanfleet, R., "Sol-Gel Synthesis And Phase Evolution Behavior Of Sterically Stabilized Nanocrystalline Zirconia" (2003). Scopus Export 2000s. 1730.
https://stars.library.ucf.edu/scopus2000/1730