Title
Absorption Anisotropy Studies Of Polymethine Dyes
Keywords
Anisotropy; Exited-state absorption; Orientation of transition dipole moments; Polymethine dye; Pump-probe
Abstract
The determination of the spectral position of the excited states and orientation of the transition dipole moments of polymethine molecules is experimentally measured using two methods: the steady-state fluorescence anisotropy method, and a two-color polarization-resolved pump-probe method. This novel use of the pump-probe method is described in detail and a comparison to the fluorescence method is given. Quantum-chemical modeling on the effects of the bridge structure in the polymethine chromophore on the linear absorption spectrum is also discussed. © 2004 Elsevier B.V. All rights reserved.
Publication Date
11-15-2004
Publication Title
Chemical Physics
Volume
306
Issue
1-3
Number of Pages
171-183
Document Type
Article
Personal Identifier
scopus
DOI Link
https://doi.org/10.1016/j.chemphys.2004.07.021
Copyright Status
Unknown
Socpus ID
5644302243 (Scopus)
Source API URL
https://api.elsevier.com/content/abstract/scopus_id/5644302243
STARS Citation
Lepkowicz, Richard S.; Cirloganu, Claudiu M.; Przhonska, Olga V.; Hagan, David J.; and Van Stryland, Eric W., "Absorption Anisotropy Studies Of Polymethine Dyes" (2004). Scopus Export 2000s. 4655.
https://stars.library.ucf.edu/scopus2000/4655