Title

Probing Many-Body Interactions In A Disordered Semiconductor Quantum Well With Electronic Two-Dimensional Fourier Transform Spectroscopy

Keywords

Coulomb interaction; Disorder; Semiconductor quantum wells; Spectroscopy

Abstract

The interplay between disorder and Coulomb interactions ubiquitously affects the properties of condensed matter systems. We examine its role in the nonlinear optical response of semiconductor quantum wells. In particular, we investigate the coherent coupling strength between exciton resonances that are spectrally split by interface fluctuations. Previous studies yielded conflicting results. In light of rising interest in semiconductor devices that rely on spatial and/or temporal coherence, we revisit this problem by applying a newly developed spectroscopy method: electronic two-dimensional Fourier transform spectroscopy (2DFTS). 2DFTS is a powerful technique for revealing the presence of coupling and for distinguishing the (coherent or incoherent) nature of such coupling, especially in complex systems with several spectrally overlapping resonances. Even the most basic information about such complex systems, including the homogeneous and inhomogeneous linewidths of various resonances, cannot be extracted reliably using conventional spectroscopic tools. In these new 2DFTS measurements, we did not observe any clear cross peaks corresponding to coherent couplings between either heavy-hole or light-hole excitons. These measurements allow us to place a quantitative upper bound on the possible coupling strength in this prototypical system. A modified mean-field theory reveals a simple yet important relation that determines how the coherent coupling strength depends on the disorder correlation length and Coulomb interaction length. © 2010 Copyright SPIE - The International Society for Optical Engineering.

Publication Date

5-3-2010

Publication Title

Proceedings of SPIE - The International Society for Optical Engineering

Volume

7600

Number of Pages

-

Document Type

Article; Proceedings Paper

Personal Identifier

scopus

DOI Link

https://doi.org/10.1117/12.840125

Socpus ID

77951568307 (Scopus)

Source API URL

https://api.elsevier.com/content/abstract/scopus_id/77951568307

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