Title

Trends In The Binding Strength Of Surface Species On Nanoparticles: How Does The Adsorption Energy Scale With The Particle Size?

Keywords

adsorption calorimetry; binding strength; metal nanoparticles; oxygen; palladium

Abstract

The binding energy of oxygen on Pd nanoparticles was measured by a direct calorimetric method as a function of the particle size. The reduced dimensionality of the Pd substrate results in two counteracting trends: an increase of the Pd-O binding strength due to a change of the local configuration of the adsorption site and a strong decrease of the Pd-O bonding due to the reduction of the cluster size. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Publication Date

5-3-2013

Publication Title

Angewandte Chemie - International Edition

Volume

52

Issue

19

Number of Pages

5175-5179

Document Type

Article

Personal Identifier

scopus

DOI Link

https://doi.org/10.1002/anie.201209476

Socpus ID

84877710994 (Scopus)

Source API URL

https://api.elsevier.com/content/abstract/scopus_id/84877710994

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