Title

Sol-gel synthesis and phase evolution behavior of sterically stabilized nanocrystalline zirconia

Authors

Authors

S. Shukla; S. Seal;R. Vanfleet

Abbreviated Journal Title

J. Sol-Gel Sci. Technol.

Keywords

sol-gel; nanocrystalline; zirconia; hydroxypropyl cellulose; XPS; steric-stabilization; CERAMIC POWDERS; TETRAGONAL ZRO2; CATALYSTS; TIO2; Materials Science, Ceramics

Abstract

Nanocrystalline as well as submicron sized, non-agglomerated, spherical ZrO2 particles have been successfully synthesized using the sol-gel technique utilizing hydroxypropyl cellulose (HPC) as a polymeric steric stabilizer. The effect of various parameters such as the ratio of molar concentration of water and alkoxide (R), the molar concentration [HPC] and the molecular weight (MWHPC) of HPC polymer as well as the calcination temperature on ZrO2 nanocrystallites size and their phase evolution behavior is systematically studied. The phase evolution behavior of nanocrystalline ZrO2 is explained and correlated with the adsorption behavior of HPC polymer on ZrO2 nanoparticles surface, which is observed to be a function of R, [HPC], MWHPC and the calcination temperature. Optimum synthesis parameters for obtaining 100% tetragonal phase in nanocrystalline ZrO2 are identified for the present sol-gel method of synthesizing nanoparticles.

Journal Title

Journal of Sol-Gel Science and Technology

Volume

27

Issue/Number

2

Publication Date

1-1-2003

Document Type

Article

Language

English

First Page

119

Last Page

136

WOS Identifier

WOS:000182923000003

ISSN

0928-0707

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