Title

Effect of acrylic acid additive on electric conductivity of polymer-derived amorphous silicon carbonitride

Authors

Authors

X. Q. Li; K. W. Wang; B. S. Ma; H. R. Hong; M. Zhang; J. L. Liu; Y. G. Wang;L. N. An

Comments

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Abbreviated Journal Title

Ceram. Int.

Keywords

Electric conductivity; Photo-polymerization; Polymer-derived amorphous; SiCN; Acrylic acid; PYROLYSIS TEMPERATURE; SICN MEMS; CERAMICS; PHOTOPOLYMERIZATION; SPECTROSCOPY; FILMS; PIEZORESISTIVITY; FABRICATION; TRANSPORT; SPECTRA; Materials Science, Ceramics

Abstract

The effect of acrylic acid additive on the electric conductivity of amorphous SiCN derived from polymeric precursor was studied. The conductivity showed to follow the Arrhenius dependence on pyrolysis temperature, but with much smaller activation energy, as compared to the unmodified SiCN. Structural analysis using Raman and XPS revealed that the size of the free-carbon clusters within the AC-modified SiCN changed with pyrolysis temperature, but the sp(2)-to-sp(3) ratio remained almost the same. The reason for the effect of AC on the carbon cluster was speculated. The mechanisms governing the conductivity behavior of the AC-modified SiCN were discussed. (C) 2015 Elsevier Ltd and Techna Group S.r.l. All rights reserved.

Journal Title

Ceramics International

Volume

41

Issue/Number

6

Publication Date

1-1-2015

Document Type

Article

Language

English

First Page

7971

Last Page

7976

WOS Identifier

WOS:000354140300100

ISSN

0272-8842

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