Authors

M. Ayouz; O. Dulieu; R. Guerout; J. Robert;V. Kokoouline

Comments

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Abbreviated Journal Title

J. Chem. Phys.

Keywords

NEGATIVE HYDROGEN-IONS; VELOCITY H-IONS; CONFIGURATION-INTERACTION; REACTION PROBABILITIES; QUANTUM DYNAMICS; GROUND-STATE; AB-INITIO; REARRANGEMENT REACTION; ROTATIONAL-EXCITATION; INELASTIC SCATTERING; Physics, Atomic, Molecular & Chemical

Abstract

A new potential energy surface for the electronic ground state of the simplest triatomic anion H-3(-) is determined for a large number of geometries. Its accuracy is improved at short and large distances compared to previous studies. The permanent dipole moment surface of the state is also computed for the first time. Nine vibrational levels of H-3(-) and 14 levels of D-3(-) are obtained, bound by at most similar to 70 and similar to 126 cm(-1), respectively. These results should guide the spectroscopic search of the H-3(-) ion in cold gases (below 100K) of molecular hydrogen in the presence of H- ions.

Journal Title

Journal of Chemical Physics

Volume

132

Issue/Number

19

Publication Date

1-1-2010

Document Type

Article

Language

English

First Page

11

WOS Identifier

WOS:000277970100022

ISSN

0021-9606

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