Title
Novel Nanoscale Ceria-Platinum Composite Electrodes For Direct Alcohol Electro-Oxidation
Keywords
Catalysis; Ceria; Direct alcohol fuel cells; Electrochemistry; Methanol; Oxidation
Abstract
A nanocrystalline Pt/CeO2 composite electrode is fabricated to study the electrochemical oxidation of methanol and ethanol. Three different methods have been developed for the preparation of the composite electrode and are compared in terms of their oxidation efficiencies. In general, all the electrode preparation methodologies show a great enhancement of the oxidation current for the alcohol. However, methods based on the electrodeposition of a ceria rich Pt matrix show the greatest effectiveness of alcohol oxidation. The enhancement of the anodic current is dependent on the particle loading and size distribution in the composite matrix. In general, ceria appears to be an effective alternative to ruthenium in direct alcohol fuel cells. © 2007 Springer Science+Business Media, LLC.
Publication Date
12-1-2007
Publication Title
Catalysis Letters
Volume
119
Issue
3-4
Number of Pages
319-326
Document Type
Article
Personal Identifier
scopus
DOI Link
https://doi.org/10.1007/s10562-007-9238-y
Copyright Status
Unknown
Socpus ID
36349035098 (Scopus)
Source API URL
https://api.elsevier.com/content/abstract/scopus_id/36349035098
STARS Citation
Díaz, Diego J.; Greenletch, Nathan; Solanki, Avni; Karakoti, Ajay; and Seal, Sudipta, "Novel Nanoscale Ceria-Platinum Composite Electrodes For Direct Alcohol Electro-Oxidation" (2007). Scopus Export 2000s. 5853.
https://stars.library.ucf.edu/scopus2000/5853