Title
Tailoring Electronic Structure Through Alloying: The Ag NCu 34-N (N = 0-34) Nanoparticle Family
Keywords
Colloid; Nanoparticles; Sensing; Zinc ion
Abstract
In this work, we report sensing of Zn 2+ ions using chitosan capped colloidal gold nanoparticles in aqueous media. The chitosan capping not just acted as an electro-static stabilizer to the colloidal gold nanoparticles, but also could bind to Zn 2+ ions if present in the solution. However, the Zn 2+ ions chelation to the chitosan capping decreased the stability of the colloidal gold hence shifted the surface plasmon peak to higher wavelengths. The extent of this red shift was found to be dependent on the concentration of the Zn 2+ ions and therefore the presence of Zn 2+ ions could be determined both qualitatively and quantitatively by analyzing the optical spectra of the chitosan capped gold nanoparticles. The sensing capability was also affected by the size of the nanoparticles, which could be tuned by adjusting the molar ratio of the reducing agent and the gold salt to the desired levels. Optical characteristics showed satisfactory results in estimating the amount of Zn 2+ ions in water. This is thus a promising method for on the spot assessment of heavy metal ion concentrations in water. © (2011) Trans Tech Publications, Switzerland.
Publication Date
1-12-2012
Publication Title
Journal of Physical Chemistry C
Volume
116
Number of Pages
281-291
Document Type
Article
Personal Identifier
scopus
DOI Link
https://doi.org/10.1021/jp208564h
Copyright Status
Unknown
Socpus ID
84855876380 (Scopus)
Source API URL
https://api.elsevier.com/content/abstract/scopus_id/84855876380
STARS Citation
Yildirim, Handan; Kara, Abdelkader; and Rahman, Talat S., "Tailoring Electronic Structure Through Alloying: The Ag NCu 34-N (N = 0-34) Nanoparticle Family" (2012). Scopus Export 2010-2014. 4933.
https://stars.library.ucf.edu/scopus2010/4933