Title

In-Depth Atomic Structure Of The Pentacene/Cu(110) Interface In The Monolayer Coverage Regime: Theory And X-Ray Diffraction Results

Abstract

The atomic structure of the pentacene/Cu(110) interface for coverages at and just below one monolayer has been determined by surface X-ray diffraction (SXRD), supported by state-of-the-art density functional theory (DFT) calculations. The in-depth sensitivity of SXRD to atom positions allows tracking the adsorption-induced distortions down to the fifth substrate layer. The main feature of the DFT model, namely, the buckling induced in the substrate, is fully confirmed by the experiment. The considerable atomic displacements which are the same for the two coverages under investigation are a signature of the strong molecule-substrate interaction, indicative of an adsorption mechanism of chemisorption type.

Publication Date

12-4-2014

Publication Title

Journal of Physical Chemistry C

Volume

118

Issue

48

Number of Pages

27815-27822

Document Type

Article

Personal Identifier

scopus

DOI Link

https://doi.org/10.1021/jp505403z

Socpus ID

84915750136 (Scopus)

Source API URL

https://api.elsevier.com/content/abstract/scopus_id/84915750136

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